- Yang, Jixiang;
- Chen, Guorui;
- Han, Tianyi;
- Zhang, Qihang;
- Zhang, Ya-Hui;
- Jiang, Lili;
- Lyu, Bosai;
- Li, Hongyuan;
- Watanabe, Kenji;
- Taniguchi, Takashi;
- Shi, Zhiwen;
- Senthil, Todadri;
- Zhang, Yuanbo;
- Wang, Feng;
- Ju, Long
ABC-stacked trilayer graphene/hexagonal boron nitride moiré superlattice (TLG/hBN) has emerged as a playground for correlated electron physics. We report spectroscopy measurements of dual-gated TLG/hBN using Fourier transform infrared photocurrent spectroscopy. We observed a strong optical transition between moiré minibands that narrows continuously as a bandgap is opened by gating, indicating a reduction of the single-particle bandwidth. At half-filling of the valence flat band, a broad absorption peak emerges at ~18 milli-electron volts, indicating direct optical excitation across an emerging Mott gap. Similar photocurrent spectra are observed in two other correlated insulating states at quarter- and half-filling of the first conduction band. Our findings provide key parameters of the Hubbard model for the understanding of electron correlation in TLG/hBN.