A host of astrophysical measurements suggest that most of the matter in the Universe is an invisible, nonluminous substance that physicists call “dark matter.” Understanding the nature of dark matter is one of the greatest challenges of modern physics and is of paramount importance to our theories of cosmology and particle physics. This text explores one of the leading hypotheses to explain dark matter: that it consists of ultralight bosons forming an oscillating field that feebly interacts with light and matter. Many new experiments have emerged over the last decade to test this hypothesis, involving state-of-the-art microwave cavities, precision nuclear magnetic resonance (NMR) measurements, dark matter “radios,” and synchronized global networks of atomic clocks, magnetometers, and interferometers. The editors have gathered leading experts from around the world to present the theories motivating these searches, evidence about dark matter from astrophysics, and the diverse experimental techniques employed in searches for ultralight bosonic dark matter.

A ferromagnetic needle is predicted to precess about the magnetic field axis at a Larmor frequency Ω under conditions where its intrinsic spin dominates over its rotational angular momentum, Nℏ≫IΩ (I is the moment of inertia of the needle about the precession axis and N is the number of polarized spins in the needle). In this regime the needle behaves as a gyroscope with spin Nℏ maintained along the easy axis of the needle by the crystalline and shape anisotropy. A precessing ferromagnetic needle is a correlated system of N spins which can be used to measure magnetic fields for long times. In principle, by taking advantage of rapid averaging of quantum uncertainty, the sensitivity of a precessing needle magnetometer can far surpass that of magnetometers based on spin precession of atoms in the gas phase. Under conditions where noise from coupling to the environment is subdominant, the scaling with measurement time t of the quantum- and detection-limited magnetometric sensitivity is t^{-3/2}. The phenomenon of ferromagnetic needle precession may be of particular interest for precision measurements testing fundamental physics.

Agreement between theoretical calculations of atomic structure and spectroscopic measurements is used to constrain possible contribution of exotic spin-dependent interactions between electrons to the energy differences between states in helium-4. In particular, constraints on dipole-dipole interactions associated with the exchange of pseudoscalar bosons (such as axions or axion-like particles) with masses 10-2"m"104eV are improved by a factor of ∼100. The first atomic-scale constraints on several exotic velocity-dependent dipole-dipole interactions are established as well.