- Liu, Shouzheng;
- Xu, Yishuai;
- Kotta, Erica C;
- Miao, Lin;
- Ran, Sheng;
- Paglione, Johnpierre;
- Butch, Nicholas P;
- Denlinger, Jonathan D;
- Chuang, Yi-De;
- Wray, L Andrew
The recent discovery of spin-triplet superconductivity emerging from a nonmagnetic parent state in UTe2 has stimulated great interest in the underlying mechanism of Cooper pairing. Experimental characterization of short-range electronic and magnetic correlations is vital to understanding these phenomena. Here we use resonant inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy (XAS), and atomic-multiplet-based modeling to shed light on the active debate between 5f26d1-based models with singlet crystal field states versus 5f3-based models that predict atomic Kramers doublets and much greater 5f itinerancy. The XAS and RIXS data are found to agree strongly with predictions for a 5f26d1-like valence electron configuration with weak intradimer magnetic correlations, and provide a context for interpreting recent investigations of the electronic structure and superconducting pairing mechanism.