A Clear Zone (CZ), the unobstructed roadside area with highly compacted soil, naturally accumulates high concentrations of pollutants from traffic activities. These pollutants are washed off by road runoff and enter waterways. In situ, treatment of polluted runoff from the CZ could not only protect water resources but also provide an opportunity to recharge groundwater. However, the soil in the CZ requires compaction, which limits the natural infiltration and treatment of road runoff. In this study, we examine whether and how amending the soil in the CZ with sand, a common bulking agent used in road design, and Expanded Shale, Clay, and Slate (ESCS) aggregates, a novel light-weight engineered bulking agent, could help treat stormwater in situ. ESCS-amended soil media infiltrated 220% more water than sand-amended soil under compaction, indicating that the addition of ESCS would make the CZ better at treating road runoff generated during high-intensity rainfall. Compared to sand-amended soil in the CZ, ESCS-amended soil provided 58% more plant-available water during prolonged drying, indicating that ESCS addition would help maintain vegetation, thereby minimizing maintenance needs. Finally, replacing sand with ESCS improved the soil capacity in the CZ to remove pollutants, including heavy metals and E. coli, indicating the performance life of ESCS-amended soil would be longer than that of sand-amended soil in the CZ. Collectively, these results indicate that the addition of ESCS as an alternative bulking agent to sand in compacted soil in the CZ could potentially treat road runoff in situ and prevent pollution originating from road infrastructure.