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Diels–Alder Construction of Regiodifferentiated meta-Amino Phenols and Derivatives
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https://doi.org/10.1021/ol4034447Abstract
Synthetic access to regiodifferentiated meta-amino phenols is described. The strategy relies upon distinct deprotonation conditions to afford regioisomeric thermodynamic and kinetic dienes that undergo a tandem Diels-Alder and retro-Diels-Alder sequence with assorted acetylenic dienophiles to afford a range of aromatic products.
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