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Studying spatio-energetic dynamics in light harvesting complex II using two-dimensional electronic-vibrational spectroscopy

  • Author(s): Lewis, NHC
  • Oliver, TAA
  • Ballottari, M
  • Gruenke, NL
  • Bassi, R
  • Fleming, GR
  • et al.
Abstract

We present two-dimensional electronic-vibrational spectra of the chlorophyll (Chl) binding protein light harvesting complex II (LHCII) from spinach, and of isolated Chl a and Chl b. We show how energy transfer from Chl b to Chl a and subsequent relaxation can be directly observed in LHCII using this multidimensional technique.

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