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Total Synthesis of (−)-Chromodorolide B
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https://doi.org/10.1021/jacs.6b00541Abstract
The first total synthesis of a chromodorolide diterpenoid is described. The synthesis features a bimolecular radical addition/cyclization/fragmentation cascade that unites butenolide and trans-hydrindane fragments while fashioning two C-C bonds and stereoselectively forming three of the ten contiguous stereocenters of chromodorolide B.
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