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Potential for Ladderane (Bio)synthesis from Oligo-Cyclopropane Precursors
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https://doi.org/10.1021/acsomega.0c03735Abstract
Quantum chemical calculations were used to determine the energetic viability of several mechanisms for formation of ladderanes from oligocyclopropanes. Pathways involving radical cations, diradicals, and carbocations were considered, and a hybrid of carbocation and radical cation pathways was predicted to have the lowest overall barrier.
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