UC Irvine

Electron spin resonance (ESR) can probe conduction electrons (CE) and local moment (LM) spin systems in different materials. A CE spin resonance (CESR) is observed in metallic systems based on light elements or with enhanced Pauli susceptibility. LM ESR can be seen in compounds with paramagnetic ions and localized d or f electrons. Here we report a remarkable and unprecedented ESR signal in the heavy-fermion superconductor β-YbAlB₄ [S. Nakatsuji et al., Nature Phys. 4, 603 (2008)] which behaves as a CESR at high temperatures and acquires characteristics of the Yb³⁺ LM ESR at low temperature. This dual behavior strikes as an in situ unique observation of the Kondo quasiparticles in a quantum critical regime. The proximity to a quantum critical point may favor the appearance of this dual character of the ESR signal in β-YbAlB₄.