- Jin, Chenhao;
- Kim, Jonghwan;
- Utama, M Iqbal Bakti;
- Regan, Emma C;
- Kleemann, Hans;
- Cai, Hui;
- Shen, Yuxia;
- Shinner, Matthew James;
- Sengupta, Arjun;
- Watanabe, Kenji;
- Taniguchi, Takashi;
- Tongay, Sefaattin;
- Zettl, Alex;
- Wang, Feng
Transition metal dichalcogenide (TMDC) materials are promising for spintronic and valleytronic applications because valley-polarized excitations can be generated and manipulated with circularly polarized photons and the valley and spin degrees of freedom are locked by strong spin-orbital interactions. In this study we demonstrate efficient generation of a pure and locked spin-valley diffusion current in tungsten disulfide (WS2)-tungsten diselenide (WSe2) heterostructures without any driving electric field. We imaged the propagation of valley current in real time and space by pump-probe spectroscopy. The valley current in the heterostructures can live for more than 20 microseconds and propagate over 20 micrometers; both the lifetime and the diffusion length can be controlled through electrostatic gating. The high-efficiency and electric-field-free generation of a locked spin-valley current in TMDC heterostructures holds promise for applications in spin and valley devices.