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Rapid Photovoltaic Device Characterization through Bayesian Parameter Estimation
- Brandt, Riley E;
- Kurchin, Rachel C;
- Steinmann, Vera;
- Kitchaev, Daniil;
- Roat, Chris;
- Levcenco, Sergiu;
- Ceder, Gerbrand;
- Unold, Thomas;
- Buonassisi, Tonio
Published Web Location
https://doi.org/10.1016/j.joule.2017.10.001Abstract
In photovoltaic (PV) materials development, the complex relationship between device performance and underlying materials parameters obfuscates experimental feedback from current-voltage (J-V) characteristics alone. Here, we address this complexity by adding temperature and injection dependence and applying a Bayesian inference approach to extract multiple device-relevant materials parameters simultaneously. Our approach is an order of magnitude faster than the cumulative time of multiple individual spectroscopy techniques, with added advantages of using device-relevant materials stacks and interface conditions. We posit that this approach could be broadly applied to other semiconductor- and energy-device problems of similar complexity, accelerating the pace of experimental research.
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