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Rational solvent molecule tuning for high-performance lithium metal battery electrolytes

2022

Yu, Zhiao;
Rudnicki, Paul E;
Zhang, Zewen;
Huang, Zhuojun;
Celik, Hasan;
Oyakhire, Solomon T;
Chen, Yuelang;
Kong, Xian;
Kim, Sang Cheol;
Xiao, Xin;
Wang, Hansen;
Zheng, Yu;
Kamat, Gaurav A;
Kim, Mun Sek;
Bent, Stacey F;
Qin, Jian;
Cui, Yi;
Bao, Zhenan
et al.

Published Web Location

https://doi.org/10.1038/s41560-021-00962-y

Creative Commons 'BY-NC-ND' version 4.0 license

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Rational solvent molecule tuning for high-performance lithium metal battery electrolytes\r
Design logic of fluorinated-DEE molecular family\r
Improved ionic transport by experimental results\r
Rationales for improved ionic conduction\r
Enhanced Li metal and oxidative stability\r
Performance of Li metal and anode-free full cells\r
Li morphology, SEI structure and cathode characterization\r
Overall evaluation of fluorinated-DEE electrolytes\r
Conclusions\r
Methods\r
Acknowledgements\r
Fig. 1 Step-by-step design principles of the fluorinated-DEE solvent family.
Fig. 2 Ionic conductivity and cycling overpotential of FDMB and fluorinated-DEE electrolytes.
Fig. 3 Theoretical and experimental study on the Li+ solvation structures and the structure–property correlations.
Fig. 4 Li metal efficiency and high-voltage stability.
Fig. 5 Full-cell performance of FDMB and fluorinated-DEE electrolytes.
Fig. 6 Li metal morphology in fluorinated-DEE electrolytes.
Fig. 7 SEI examination in fluorinated-DEE electrolytes.
Fig. 8 Summary and overall evaluation of fluorinated-DEE electrolytes.

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