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Self-optimizing, highly surface-active layered metal dichalcogenide catalysts for hydrogen evolution

2017

Liu, Yuanyue;
Wu, Jingjie;
Hackenberg, Ken P;
Zhang, Jing;
Wang, Y. Morris;
Yang, Yingchao;
Keyshar, Kunttal;
Gu, Jing;
Ogitsu, Tadashi;
Vajtai, Robert;
Lou, Jun;
Ajayan, Pulickel M;
Wood, Brandon C;
Yakobson, Boris I
et al.

Published Web Location

https://doi.org/10.1038/nenergy.2017.127

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Self-optimizing, highly surface-active layered metal dichalcogenide catalysts for hydrogen evolution
Understanding the surface activity of MX2
Experimental verification
Conclusion
Methods
Figure 1 Electronic origin of MX2 surface activity and the derived descriptor (LUS) for catalysts screening.
Figure 2 HER electrocatalysis on H-TaS2 and H-NbS2.
Figure 3 Morphological evolution of H-TaS2 following cycling.
Figure 4 Chemical intactness and origin of self-optimizing behaviour.
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