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New heavy-fermion system, NpBe13, with a comparison to UBe13 and PuBe13

Abstract

We have prepared single crystals of NpBe13, Np0.68U0.32Be13, and PuBe13 and measured their resistivity, susceptibility, and specific heat down to low temperatures. NpBe13 has an itinerant-electron magnetic transition at 3.4 K, with a large temperature-dependent specific heat above this transition that is quite similar to that observed in the heavy-fermion superconductor UBe13 and a (T=0) of approximately 900 mJ/mole K2. PuBe13 may be described as a Kondo-type system, with certain inconsistencies. The data are compared to results for UBe13 and are consistent with a narrow f band at the Fermi energy in UBe13 moving lower in energy with the addition of f electrons in heavier actinide elements to create a Kondo resonance by PuBe13. © 1984 The American Physical Society.

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