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Cobalt Catalysis for Enantioselective Cyclobutanone Construction
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https://doi.org/10.1021/jacs.7b05327Abstract
Over the past 40 years, intramolecular hydroacylation has favored five-membered rings, in preference to four membered rings. Herein, we report a catalyst derived from earth-abundant cobalt that enables preparation of cyclobutanones, with excellent regio-, diastereo-, and enantiocontrol, under mild conditions (2 mol % catalyst loading and as low as 50 °C).
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