UC Berkeley

Quantum processors based on superconducting circuitry have reached the scale of hundreds of qubits and demonstrated computational capabilities that challenge state-of-the-art classical methods for carefully designed problems. Despite these advances, fundamental questions persist over how to best improve and scale the computational power of this emerging technology. Most transmon-based quantum processors encode information in two-level systems, or qubits, leaving the rich multilevel structure of the transmon largely unexploited. In this thesis, we demonstrate how the capabilities of these devices can be meaningfully extended by harnessing this intrinsic multilevel structure to encode qudits — d-level quantum systems that access a larger and more connected Hilbert space than their qubit counterparts. We begin by demonstrating universal single-qudit operation before turning to microwave-activated entanglement to realize scalable two-qudit gates. We present a high-fidelity, fully entangling two-qutrit CZ gate based on a novel tunable cross-Kerr mechanism. We further explore two-qudit gates that selectively entangle subspaces of the full Hilbert space via two-photon multipartite Raman transitions, employing these operations to generate large entangled states across a transmon array. To address the noisy nature of near-term qudit computation, we introduce and characterize error suppression techniques for qudit circuits, including dynamical decoupling and quantum error mitigation. We then synthesize these directions by exploring simulations of quantum systems that have innate multilevel interactions and are therefore well tailored to qudit operation. First we investigate digital quantum simulations of collective neutrino oscillations and the spin-1 truncated Abelian Higgs model, finding error mitigation methods critical for improving circuit performance. Finally, out of equilibrium --- or Floquet --- spin-1 systems are realized using an array of 15 superconducting qutrits to probe a novel Z3 discrete time crystalline (DTC) phase of matter with intrinsically chiral interactions. This DTC result demonstrates that native qudit hardware provides powerful access to non-equilibrium phases rooted in higher discrete symmetries, opening a route to a broader landscape of dynamical orders beyond the Z2 Ising paradigm.