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Open Access Publications from the University of California

Conductive Polymer Binder-Enabled SiO-SnxCoyCz Anode for High-Energy Lithium-Ion Batteries.

  • Author(s): Zhao, Hui;
  • Fu, Yanbao;
  • Ling, Min;
  • Jia, Zhe;
  • Song, Xiangyun;
  • Chen, Zonghai;
  • Lu, Jun;
  • Amine, Khalil;
  • Liu, Gao
  • et al.

A SiOSnCoC composite anode is assembled using a conductive polymer binder for the application in next-generation high energy density lithium-ion batteries. A specific capacity of 700 mAh/g is achieved at a 1C (900 mA/g) rate. A high active material loading anode with an areal capacity of 3.5 mAh/cm(2) is demonstrated by mixing SiOSnCoC with graphite. To compensate for the lithium loss in the first cycle, stabilized lithium metal powder (SLMP) is used for prelithiation; when paired with a commercial cathode, a stable full cell cycling performance with a 86% first cycle efficiency is realized. By achieving these important metrics toward a practical application, this conductive polymer binder/SiOSnCoC anode system presents great promise to enable the next generation of high-energy lithium-ion batteries.

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